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1 article(s) from Agraït, Nicolás

Single-molecule conductance of a chemically modified, π-extended tetrathiafulvalene and its charge-transfer complex with F₄TCNQ

Raúl García,
M. Ángeles Herranz,
Edmund Leary,
M. Teresa González,
Gabino Rubio Bollinger,
Marius Bürkle,
Linda A. Zotti,
Yoshihiro Asai,
Fabian Pauly,
Juan Carlos Cuevas,
Nicolás Agraït and
Nazario Martín

Beilstein J. Org. Chem. 2015, 11, 1068–1078, doi:10.3762/bjoc.11.120

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Graphical Abstract

Figure 1: Depictions of 9,10-bis(1,3-dithiol-2-ylidene)-9,10-dihydroanthracene (exTTF) in the (a) neutral for...

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Scheme 1: Synthetic route to the target exTTF-based molecular wire 5.

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Figure 2: Cyclic voltammograms of compound 5 and pristine exTTF (at concentrations of approximately 0.2 mM) u...

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Figure 3: 2D histograms resulting from break junction experiments on an unmodified gold sample (a), OPE3-dith...

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Figure 4: 2D histograms corresponding to compound 5 after exposing a gold substrate to the solution of the co...

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Figure 5: 2D histograms corresponding to compound 5 after exposing a gold substrate to a solution of the comp...

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Figure 6: a) Examples of individual G(z) traces showing clear conductance plateaus. b–e) 2D histograms corres...

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Figure 7: Frontier orbitals of compound 5 in the gas phase.

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Figure 8: Top a) and hollow b) binding geometries of 5 to a gold cluster in metal–molecule–metal junctions.

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Figure 9: Transmission as a function of energy for the top and hollow binding geometries.

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Published 24 Jun 2015

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Single-molecule conductance of a chemically modified, π-extended tetrathiafulvalene and its charge-transfer complex with F4TCNQ

Single-molecule conductance of a chemically modified, π-extended tetrathiafulvalene and its charge-transfer complex with F₄TCNQ